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The research on amorphous coatings for future GW detectors Francesco Piergiovanni University of Urbino - INFN Firenze on behalf of the Virgo Collaboration Thermal Noise It characterizes each dissipative mechanical system at thermal


  1. The research on amorphous coatings for future GW detectors Francesco Piergiovanni University of Urbino - INFN Firenze on behalf of the Virgo Collaboration

  2. Thermal Noise • It characterizes each dissipative mechanical system at thermal equilibrium • It’s produced by irreversible processes with typical time constants and activation energies • Same mechanism produces energy dissipation and thermal fluctuation Fluctuation-Dissipation Theorem Mechanical dissipation is quantified by the loss angle 𝑇 𝑦 𝜕 = 4𝑙 𝐶 𝑈 Dissipation 𝐹 𝑚𝑝𝑡𝑢 𝑞𝑓𝑠 𝑑𝑧𝑑𝑚𝑓 𝜕 2 𝑆𝑓[𝑍 𝜕 ] 𝜚 𝜕 = 2𝜌𝐹 𝑡𝑢𝑝𝑠𝑓𝑒 ( Callen, Welton 1951) Fluctuation 𝜚 𝜕 = 1/𝑅 @ resonances Thermal noise can be reduced: • low temperature • low dissipation material 2 TAUP 2019 - TOYAMA

  3. The origin of the TN amorphous materials • In Two Level System (TLS): metastable states are separated 𝜐 ∝ 𝜐 0 Δ exp 𝑊/ 𝑙 𝑐 𝑈 Gilroy & Phillips by an energy barrier 𝑊 : barrier high Philosophical Magazine B (1981) • Transitions between the two levels explain the anelastic behavior of amorphous materials • Only transitions with a relaxation time of the same order of the period of the strain wave propagating in the material produce mechanical losses. At room temperature ( 300 𝐿 ) only TLS with 𝑊 ≈ 0.5𝑓𝑊 are relevant 𝜐 Too fast relaxation 𝜐 Too slow relaxation 𝜐 Relaxation producing losses Dove et al. Mineralogical Magazine (2000) 3 TAUP 2019 - TOYAMA

  4. Coating In GW detectors SiO2 thinner layer (cap) • Alternate layers of transparent materials with different Ta2O5-TiO2 layer N doublets index of refraction (Bragg reflection). ~6 µm SiO2 layer Ta2O5-TiO2 thicker layer • Impedance mismatch and interference produce high coefficient of reflectivity. 35 cm • Its structure is not compact as the substrate. • 5 𝜈𝑛 of coating produces more thermal noise than 20 cm 20 𝑑𝑛 of substrate. 40 kg 2 2𝑂 𝑜 𝐼 − 1 Aasi J et al. 2015 Classical and Quantum Gravity 32 𝑜 𝑀 𝑆 = 𝑠 2 = Acernese F et al. 2015 Classical and Quantum Gravity 32 2𝑂 𝑜 𝐼 + 1 𝑜 𝑀 4 TAUP 2019 - TOYAMA

  5. Coating thermal noise Advanced Virgo Coating Thermal Noise (CTN) limits the detection band in the « bucket » (middle frequencies) which is the most sensitive region of the Advanced and the future Advanced+ GW detectors 5 TAUP 2019 - TOYAMA

  6. Coating thermal noise (CTN) Coating thermal noise (CTN) contribution goes like: 𝑇 𝑦 𝜕 ∝ 𝑈 𝑒 𝑥 2 𝜚 𝐷 Research to reduce CTN involves: • enlarging the laser beam size 𝑥 ; • minimizing the overall coating thickness ( 𝑒 ) increasing the contrast between the high and the low refractive index materials in Bragg reflector; • finding new materials-techniques for reducing the coating loss angle 𝜚 𝐷 . 6 TAUP 2019 - TOYAMA

  7. The Virgo Coating R&D activities Sysnthesis: Modeling: ✓ Coating deposition ✓ Structure ✓ Heat treatments ✓ TLS relaxations Macroscopic Microscopic characterization: characterization: ✓ Loss angle measurements ✓ TEM, SEM ✓ Optical characterization ✓ Raman, Brillouin ✓ Dielectric response ✓ XRD, XPS, XAS ✓ Elastic constants ✓ AFM ✓ Density 7 TAUP 2019 - TOYAMA

  8. The Virgo Coatings R&D Formed on January 2017 Collaboration ● LMA ♦ IBS HighT, IAD ● PADOVA ● GENOVA ♦ GeNS [300-10] K ♦ FEA ♦ Mag. Sputtering ♦ Ellipsometry ♦ Optical metrology ♦ XRD High T ♦ Optical properties ♦ AFM, XPS LMA ● g-MAG ♦ Raman ● URBINO ♦ Pulsed Laser Dep. ♦ Rapid Th. Annealing ♦ GeNS Cryo GENOVA PADOVA g-MAG ♦ Raman, Brillouin ♦ FEA ♦ Physics of Glasses URBINO ♦ Molecular Dynamics PISA ● PERUGIA-CAMERINO ● PISA ♦ Cantilevers & GeNS Cryo PERUGIA ♦ Physics of Glasses VIRGO ♦ Study of the crystallization processes ♦ Brillouin, Raman ROMA 2 ♦ Physics of deposition and ● ROMA 2 ♦ SEM, XRD, XAS ultrastable glasses ♦ Laser Polishing ♦ Molecular Dynamics and Modelling ♦ GeNS 300K 1’’ ♦ Calorimetry and Dielectric response ROMA 1 ♦ FEA and AFM ♦ XPS SALERNO ♦ Sample production ♦ Ellipsometry SANNIO ♦ Characterization ● SALERNO/SANNIO ● ROMA 1 ♦ IAD ♦ Structural Other groups (from KAGRA and ♦ SEM,TEM,AFM and XRD characterization ♦ nanolayered composites ♦ Thermobalance Belgium) are interested to join Credits: G. Cagnoli and Mie-metamaterials 8

  9. The Virgo Coating R&D research lines Oxides ● Materials Deposition Mixing ● ● High Temperature High Index ● ● Nano-layering Silica Glasses ‒ High index ‒ Low index Nitrides ● BETTER ‒ HR stack Fluorides ● COATING High Coordination ● Number Glasses SiN, GaN, SiC, etc Post-deposition Origin of absorption ● ● Annealing Absorption and treatments Loss measurement ● Metrology ● Outgassing and protocol chemical status Thermo-elastic ● ● Controlled effect crystallization O5 horizon, CRD project accepted by funding agencies Beyond O5 9 TAUP 2019 - TOYAMA

  10. Updated measurement of current coatings 𝑈𝑏 2 𝑃 5 𝑈𝑗𝑃 2 : 𝑈𝑏 2 𝑃 5 𝜚 𝑑 (𝑔) = 𝑏 𝑔 𝑐 𝜚 𝑑 𝑔 = 𝑏 𝑔 𝑐 + 𝜗 𝑒 𝜚 𝑓 𝑇𝑗𝑃 2 𝜚 𝑑 = 𝑏 𝑔 𝑐 Cagnoli et al. PLA (2018), M. Granata, OIC 2019 Refractive index: ቊ 𝑜 𝐼 = 2.09 𝑜 𝑀 = 1.45 Extinction coeff.: 𝑙 ≈ 10 −7 10 TAUP 2019 - TOYAMA

  11. Oxide mixtures recap High refractive index 𝑂𝑐 2 𝑃 5 500°C 𝑈𝑏 2 𝑃 5 500°𝐷 𝑈𝑗𝑃 2 : 𝑈 𝑏2 𝑃 5 500°C 𝑈𝑗𝑃 2 : 𝑈𝑏 2 𝑃 5 400 °C 𝑎𝑠𝑃 2 : 𝑈𝑏 2 𝑃 5 700 °C Post-deposition annealing temperature are reported 𝑇𝑗𝑃 2 500°𝐷 𝑇𝑗𝑃 2 900°𝐷 Low refractive index Granata et al. Optical Interference Coatings Conference (OIC) 2019 11 TAUP 2019 - TOYAMA

  12. Annealing Amato et al. J. Phys Conf. Ser. 957 (2018) Granata et al Phys. Rev. Mater. 2 (2018) SiO 2 𝑇𝑗𝑃 2 IBS GC – not annealed – IBS SPECTOR – annealed – fused silica – bulk – 12 TAUP 2019 - TOYAMA

  13. Deposition parameters (IBS coating) as deposited annealed 𝐻𝑠𝑏𝑜𝑏𝑢𝑏 𝑓𝑢 𝑏𝑚, 𝑗𝑜 𝑞𝑠𝑓𝑞𝑏𝑠𝑏𝑢𝑗𝑝𝑜 𝐵𝑛𝑏𝑢𝑝 𝑓𝑢 𝑏𝑚, 𝐾. 𝑄ℎ𝑧𝑡. 𝐷𝑝𝑜𝑔. 𝑇𝑓𝑠. 957 (2018) erasing effect SPECTOR 𝑈𝑏 2 𝑃 5 ✓ Films deposited with different DIBS coaters (at different rates) show GC different loss angles structural limit? ✓ Slower is the deposition, lower the dissipation as deposited annealed ✓ A sort of erasing effect of the SPECTOR annealing is visible, which is more evident for the tantala 𝑇𝑗𝑃 2 GC coating 13 TAUP 2019 - TOYAMA

  14. Absorption vs mechanical losses Urbach tail: broadening in the band-gap absorption edge especially visible in poor crystallin ✓ A strong correlation and amorphous material, related to thermal and between 𝐹 𝑉 and structural disorder mechanical losses has 𝛽 𝐹 ∝ 𝑓 𝐹/𝐹 𝑉 been found Urbach energy Absorption coefficient ✓ Different materials show the same behavior Ellipsometry ✓ Rapid estimation of mechanical losses Amato et al. ✓ Extend the range of structural analysis arXiv:1903.06094 Photon energy (eV) 14 TAUP 2019 - TOYAMA

  15. Modelling: Molecular Dynamics MD-DMS: Molecular Dynamics simulation of Dynamical Mechanical Spectroscopy • A theory-independent method: the only ingredient is the interatomic potential of the specific glassy system ( 𝑈𝑏 2 𝑃 5 , 𝑇𝑗𝐷 in progress) • Mechanical losses are computed by the dephasing btw applied oscillating strain and the resulting stress • Simulation frequency range is GHz to THz , but the frequency power law is compatible with what has been experimentally found in acoustic band • MD-DMS and experimental results, 𝑈𝑏 2 𝑃 5 are in good agreement MD-DMS makes possible a rapid evaluation of mechanical properties of new materials Puosi et al. in preparation Puosi 10th Einstein Telescope Symposium 2019 15 TAUP 2019 - TOYAMA

  16. New materials Granata et al. Optical Interference Coatings Conference (OIC) 2019 IBS coatings Amato et al. Journal of Physics: Conf. Series 957 (2018) Nitrides: 𝑇𝑗𝑂 𝑦 is a promising high index material 𝑈𝑏 2 𝑃 5 • Mechanical losses about 3x better than 𝑈𝑏 2 𝑃 5 issues • Refractive index slightly lower than 𝑈𝑏 2 𝑃 5 𝑇𝑗𝑂 𝑦 • Extinction coefficient more than 10x larger!!! 𝑁𝑕𝐺 2 as deposited Fluorides: 𝑁𝑕𝐺 2 and 𝐵𝑚𝐺 3 𝑁𝑕𝐺 2 400°C • lower refractive index than silica Bischi et al. poster GWADW 2019 issues • Higher mechanical losses than silica 𝑇𝑗𝑃 2 500°𝐷 (at least at room T) 𝑇𝑗𝑃 2 900°𝐷 16 TAUP 2019 - TOYAMA

  17. Nano-layered coating deposition • Post-deposition annealing largely improves coating mechanical characteristics. • Maximum annealing temperature is limited by the beginning of the film crystallization (i.e. T max ≈ 300 °𝐷 for 𝑈𝑗𝑃 2 ) • In nano-layered films crystallization is frustrated by the size of the layers, higher annealing temperature is allowed TiO 2 /SiO 2 stack TiO 2 = 1.8 𝑜𝑛 𝑦 38 SiO 2 = 3.6 𝑜𝑛 𝑦 37 TiO 2 = 7.36 𝑜𝑛 𝑦 10 SiO 2 = 4.32 𝑜𝑛 𝑦 9 Kuo et al., Opt. Lett.44, 247-250 (2019); Chao et al., 41 st PIERS 2019; Principe, Opt. Express 23, 10938-10956 (2015) 17 TAUP 2019 - TOYAMA

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