n TTC Topical Workshop -RF superconductivity: Pushing Cavity - - PowerPoint PPT Presentation

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n TTC Topical Workshop -RF superconductivity: Pushing Cavity - - PowerPoint PPT Presentation

arXiv:1711.03077 To be published in Physical Review B n TTC Topical Workshop -RF superconductivity: Pushing Cavity Performance Limits Fermilab, IL, USA (2017) 1 The surface resistance of an SRF cavity is usually written as the summation of


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n TTC Topical Workshop -RF superconductivity: Pushing Cavity Performance Limits Fermilab, IL, USA (2017)

arXiv:1711.03077 To be published in Physical Review B

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The surface resistance of an SRF cavity is usually written as the summation of

𝑆𝑁𝐢 : Mattis-Bardeen surface resistance

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𝑆𝑁𝐢 : Mattis-Bardeen surface resistance π‘†π‘π‘’β„Žπ‘“π‘ π‘‘ : other than the above

Damaged layer Metallic sub-oxide Subgap states Dielectric losses

etc

π‘†π‘”π‘šπ‘£π‘¦ : trapped flux contribution

The surface resistance of an SRF cavity is usually written as the summation of

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𝑆𝑁𝐢 : Mattis-Bardeen surface resistance π‘†π‘π‘’β„Žπ‘“π‘ π‘‘ : others

Damaged layer Metallic sub-oxide Subgap states Dielectric losses

etc

π‘†π‘”π‘šπ‘£π‘¦ : trapped flux contribution

The surface resistance of an SRF cavity is usually written as the summation of

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𝑆𝑁𝐢 π‘†π‘π‘’β„Žπ‘“π‘ π‘‘

Damaged layer Metallic sub-oxide Subgap states Dielectric losses

etc

π‘†π‘”π‘šπ‘£π‘¦ Rs =RMB+Rflux+Rothers

The surface resistance of an SRF cavity is usually written as the summation of

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Today, Rflux can be substantially reduced by cooling down a cavity with a large temperature gradient.



  • A. Romanenko, et al., Appl. Phys. Lett. 105

105, 234103 (2014). 

  • S. Posen et al., J. Appl. Phys. 119

119, 213903 (2016) 

  • S. Huang, T. Kubo, and R. Geng, Phys. Rev. Accel. Beams 19

19, 082001 (2016)

Rs =RMB+Rflux+Rothers 𝑆𝑁𝐢 π‘†π‘π‘’β„Žπ‘“π‘ π‘‘

Damaged layer Metallic sub-oxide Subgap states Dielectric losses

etc

π‘†π‘”π‘šπ‘£π‘¦

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Today, Rflux can be substantially reduced by cooling down a cavity with a large temperature gradient.



  • A. Romanenko, et al., Appl. Phys. Lett. 105

105, 234103 (2014). 

  • S. Posen et al., J. Appl. Phys. 119

119, 213903 (2016) 

  • S. Huang, T. Kubo, and R. Geng, Phys. Rev. Accel. Beams 19

19, 082001 (2016)

Understanding this part is is becoming im important more and more!

Rs =RMB+Rflux+Rothers 𝑆𝑁𝐢 π‘†π‘π‘’β„Žπ‘“π‘ π‘‘

Damaged layer Metallic sub-oxide Subgap states Dielectric losses

etc

π‘†π‘”π‘šπ‘£π‘¦

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Today, Rflux can be substantially reduced by cooling down a cavity with a large temperature gradient.



  • A. Romanenko, et al., Appl. Phys. Lett. 105

105, 234103 (2014). 

  • S. Posen et al., J. Appl. Phys. 119

119, 213903 (2016) 

  • S. Huang, T. Kubo, and R. Geng, Phys. Rev. Accel. Beams 19

19, 082001 (2016)

Would contain in information

  • n the meaning of surface

processing recipes.

Rs =RMB+Rflux+Rothers 𝑆𝑁𝐢 π‘†π‘π‘’β„Žπ‘“π‘ π‘‘

Damaged layer Metallic sub-oxide Subgap states Dielectric losses

etc

π‘†π‘”π‘šπ‘£π‘¦

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Rs =RMB+Rflux+Rothers

Based on the BCS theory we calc lculate Rs Rs sim imultaneously taking in into account both the contrib ibutio ions.

𝑆𝑁𝐢 π‘†π‘π‘’β„Žπ‘“π‘ π‘‘

Damaged layer Metallic sub-oxide Subgap states Dielectric losses

etc

π‘†π‘”π‘šπ‘£π‘¦

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Structures, parameters, and theoretical tool

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superconductors with im imperfect surface

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superconductors with im imperfect surface 𝑒 πœπ‘œ

Conductance

πœπ‘‘ 𝑆𝐢

Interface resistance

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superconductors with im imperfect surface 𝑒 πœπ‘œ

Conductance

πœπ‘‘ 𝑆𝐢

Interface resistance

These structures model realistic surfaces of superconducting materials which can contain

  • xide layers, absorbed impurities or

nonstoichiometric composition.

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Theoretical tool

We use the quasiclassical theory in the diffusive limit.  Self-consistency condition  Usadel equation  Boundary conditions

  • K. D. Usadel, Phys. Rev. Lett. 25, 507 (1970).
  • M. Yu. Kuprianov and V. F. Lukichev, Sov. Phys. JETP 67, 1163 (1988).

It is convenient to define the following dimensionless parameters:

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Theoretical tool

We use the quasiclassical theory in the diffusive limit.  Self-consistency condition  Usadel equation  Boundary conditions

  • K. D. Usadel, Phys. Rev. Lett. 25, 507 (1970).
  • M. Yu. Kuprianov and V. F. Lukichev, Sov. Phys. JETP 67, 1163 (1988).

It is convenient to define the following dimensionless parameters:

𝛽 = π‘‚π‘œ 𝑂𝑑 𝑒 πœŠπ‘‘ = 0.05

(when d = 1nm, πœŠπ‘‘ = 20nm, and π‘‚π‘œ = 𝑂𝑑)

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Theoretical tool

We use the quasiclassical theory in the diffusive limit.  Self-consistency condition  Usadel equation  Boundary conditions

  • K. D. Usadel, Phys. Rev. Lett. 25, 507 (1970).
  • M. Yu. Kuprianov and V. F. Lukichev, Sov. Phys. JETP 67, 1163 (1988).

It is convenient to define the following dimensionless parameters:

𝛽 = π‘‚π‘œ 𝑂𝑑 𝑒 πœŠπ‘‘ = 0.05

(when d = 1nm, πœŠπ‘‘ = 20nm, and π‘‚π‘œ = 𝑂𝑑)

𝛾 = 4𝑓2 ℏ π‘†πΆπ‘‚π‘œΞ”π‘’ = 16𝑒 𝜊0 𝑆𝐢 π‘†πΏπœ‡πΊ

2 ~

𝑆𝐢 10βˆ’14Ξ©m2

(when d = 1nm, 𝜊0 = 40nm)

For example, RB of YBCO/Ag obtained in [J. W. Ekin et al., Appl. Phys. Lett. 62, 369 (1993)] is RB~ 10-13-10-12Ξ©m2, which yields Ξ²~10-100.

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Theoretical tool

We use the quasiclassical theory in the diffusive limit.

Normal and anomalous Quasiclassical Matsubara Green functions

 Self-consistency condition  Usadel equation  Boundary conditions

  • K. D. Usadel, Phys. Rev. Lett. 25, 507 (1970).
  • M. Yu. Kuprianov and V. F. Lukichev, Sov. Phys. JETP 67, 1163 (1988).
  • T. Matsubara, Prog. Theor. Phys. 14, 351 (1955).

It is convenient to define the following dimensionless parameters:

Penetration depth

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Theoretical tool

We use the quasiclassical theory in the diffusive limit.

Normal and anomalous Quasiclassical Matsubara Green functions

 Self-consistency condition  Usadel equation  Boundary conditions

Retarded normal and anomalous Quasiclassical Green functions

Density of states and surface resistance

  • K. D. Usadel, Phys. Rev. Lett. 25, 507 (1970).
  • M. Yu. Kuprianov and V. F. Lukichev, Sov. Phys. JETP 67, 1163 (1988).
  • T. Matsubara, Prog. Theor. Phys. 14, 351 (1955).

It is convenient to define the following dimensionless parameters:

Penetration depth

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Density of States

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DOS of Normal conductor

Density of states

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DOS of Normal conductor DOS of BCS superconductor

Density of states

DOS of BCS superconductor

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DOS of Normal conductor DOS of BCS superconductor

BCS superconductor Normal conductor

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BCS superconductor Normal conductor

DOS of Normal conductor DOS of BCS superconductor

N-side DOS S-side DOS

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? ?

DOS of Normal conductor DOS of BCS superconductor

N-side DOS S-side DOS

The proximity effect changes DOS BCS superconductor Normal conductor

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N-side DOS

𝛽 = 0.05

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N-side DOS

𝛽 = 0.05

minigap

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N-side DOS S-side DOS

𝛽 = 0.05 𝛽 = 0.05

minigap

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N-side DOS S-side DOS

𝛽 = 0.05 Ξ“=0.05 𝛽 = 0.05 Ξ“=0.05

Taking into account a finite quasi particle life time (𝜁 β†’ 𝜁 + 𝑗Γ) smears out the cusps.

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DOS for the right figure (SC with a surface layer of gradually reduced BCS pairing constant) can also be calculated.

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Temperature dependence of penetration Depth

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Without subgap states

Exponential T dependence at any temperature

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Effect of subgap states Without subgap states π‘ˆ β‰ͺ π‘ˆ

𝑑

Exponential T dependence at any temperature quadratic T dependence at a low temperature

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Surface Resistance

(1)Ideal surface without subgap states (2)Ideal surface with subgap states (3)normal thin layer on the surface

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Surface Resistance

(1)Ideal surface without subgap states (2)Ideal surface with subgap states (3)normal thin layer on the surface

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gap Quasiparticles

T→0

DOS

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As T decreases, a number of quasiparticles exponentially decrease.

gap Quasiparticles

𝑆𝑑 ∝ π‘“βˆ’ βˆ†

π‘™π‘ˆ β†’ 0

T→0

T β†˜

gap

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As T decreases, a number of quasiparticles exponentially decrease.

gap Quasiparticles

T=0

𝑆𝑑 ∝ π‘“βˆ’ βˆ†

π‘™π‘ˆ β†’ 0

(𝑆𝑗 = 0)

T→0

T β†˜ T β†˜

gap gap

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Mattis-Bardeen

Typical behavior of Nb cavities

𝑆𝑁𝐢~𝑓

βˆ’ βˆ† π‘™πΆπ‘ˆ

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Surface Resistance

(1)Ideal surface without subgap states (2)Ideal surface with subgap states (3)normal thin layer on the surface

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Subgap states Quasiparticles

DOS

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Subgap states Quasiparticles Subgap states Quasiparticles

T β†˜

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Even at T→0, quasiparticles can be excited by the microwave field when finite subgap states exist.

Subgap states Quasiparticles

T→0

Subgap states Quasiparticles

T β†˜ T β†˜

Subgap states

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Even at T→0, quasiparticles can be excited by the microwave field when finite subgap states exist.

Subgap states Quasiparticles

T→0

Subgap states Quasiparticles

T β†˜ T β†˜

Subgap states

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examples

Ξ“ Ξ” = 0.06

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examples

Ξ“ Ξ” = 0.06 Ξ“ Ξ” = 0.03

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examples

Ξ“ Ξ” = 0.06 Ξ“ Ξ” = 0.03 Ξ“ Ξ” = 0.01

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examples

Ξ“ Ξ” = 0.06 Ξ“ Ξ” = 0.03 Ξ“ Ξ” = 0.01

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Ξ“ Ξ” =

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Ξ“ Ξ” =

As Ξ“ increases, the residual resistance 𝑆𝑗 increases.

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Ξ“ Ξ” =

At this region, 𝑆𝑑 decreases as Ξ“ increases.

Ξ“ Ξ” = 0.06 Ξ“ Ξ” = 0.03 Ξ“ Ξ” = 0.01

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𝑆𝑑~ ΰΆ± π‘’πœ— 𝑂 πœ— 𝑂(πœ— + β„πœ•)π‘“βˆ’πœ—/π‘™π‘ˆ

Why does Rs decrease as Ξ“ increases?

𝑆𝑑 ∝ ln π‘™π‘ˆ β„πœ•

Since we have

  • A. Gurevich, Phys. Rev. Lett. 113, 087001 (2014)
  • A. Gurevich, Supercond. Sci. Technol. 30, 034004 (2017)
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𝑆𝑑~ ΰΆ± π‘’πœ— 𝑂 πœ— 𝑂(πœ— + β„πœ•)π‘“βˆ’πœ—/π‘™π‘ˆ

Why does Rs decrease as Ξ“ increases?

𝑆𝑑 ∝ ln π‘™π‘ˆ β„πœ•

Since we have

Ξ“ Ξ” = 0.01

𝑆𝑑 ∝ ln π‘™π‘ˆ Ξ“

>

  • A. Gurevich, Phys. Rev. Lett. 113, 087001 (2014)
  • A. Gurevich, Supercond. Sci. Technol. 30, 034004 (2017)
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Ξ“ Ξ” = 0.06 Ξ“ Ξ” = 0.01

𝑆𝑑~ ΰΆ± π‘’πœ— 𝑂 πœ— 𝑂(πœ— + β„πœ•)π‘“βˆ’πœ—/π‘™π‘ˆ

Why does Rs decrease as Ξ“ increases?

𝑆𝑑 ∝ ln π‘™π‘ˆ β„πœ• 𝑆𝑑 ∝ ln π‘™π‘ˆ Ξ“

>

Since we have

>

DOS broadening can reduce Rs

  • A. Gurevich, Phys. Rev. Lett. 113, 087001 (2014)
  • A. Gurevich, Supercond. Sci. Technol. 30, 034004 (2017)

Ξ“ Ξ” = 0

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Ξ“ Ξ” =

At this region, 𝑆𝑑 decreases as Ξ“ increases. This comes from DOS broadening.[A. Gurevich, Phys. Rev.

  • Lett. 113, 087001 (2014)]

Ξ“ Ξ” = 0.06 Ξ“ Ξ” = 0.03 Ξ“ Ξ” = 0.01

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Surface Resistance

(1)Ideal surface without subgap states (2)Ideal surface with subgap states (3)normal thin layer on the surface

As seen in the above, DOS is broaden due to proximity effect. Thus we can expect Rs can be reduced by the same mechanism as before: Rs reduction by the broadening of DOS peak.

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Subgap states

N S

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Subgap states

N S

T β†˜

N S

T→0

Even at T→0, quasiparticles can be excited by the microwave field when finite subgap states exist.

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Subgap states

N S

T β†˜

N S

T→0

Even at T→0, quasiparticles can be excited by the microwave field when finite subgap states exist.

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Rs as functions of T-1

𝛾 =

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𝛾 = Similar as the ideal surface with subgap states

Rs as functions of T-1

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𝛾 = Similar as the ideal surface with subgap states

The slope is changed to that corresponding to the minigap

Rs as functions of T-1

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𝛾 = Similar as the ideal surface with subgap states

The slope is changed to that corresponding to the minigap N and S are decoupled. The residual resistance is given by normal N.

Rs as functions of T-1

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𝛾 =

Rs as functions of T-1

Extrapolating the results

  • btained in a limited

temperature window may lead to a wrong conclusion. e.g. At Ξ”/kT < 10, the curves for Ξ²=4 and 30 are nearly the same: the traditional fitting based on Rs=RMB+Ri would suggest Ri at Ξ²=30, while their actual T dependence are much different at a lower T.

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𝛾 =

Rs as functions of T-1

𝛾 =

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Ξ“ = Ξ“ =

Rs as functions of Ξ² for different T

Ξ“ = Ξ“ =

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Ξ“ = Ξ“ =

Rs as functions of Ξ² for different T

Ξ“ = Ξ“ =

The minimum in Rs(Ξ²) mainly results from interplay of two effects. The first effect which causes Rs to increase with Ξ² is rather transparent: as the barrier parameter Ξ² increases the proximity-induced superconductivity in N layer weakens, so the RF dissipation and Rs increase.

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Ξ“ = Ξ“ =

Rs as functions of Ξ² for different T

Ξ“ = Ξ“ =

The minimum in Rs(Ξ²) mainly results from interplay of two effects. The first effect which causes Rs to increase with Ξ² is rather transparent: as the barrier parameter Ξ² increases the proximity-induced superconductivity in N layer weakens, so the RF dissipation and Rs increase. The second effect which causes the initial decrease of Rs with Ξ² results from the change in DOS around N layer. A moderate broadening of the gap peaks in N(Ξ΅) eliminates the BCS logarithmic divergence at Ο‰β†’0 and reduces Rs .

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Ξ“ = Ξ“ =

Rs as functions of Ξ² for different T

Ξ“ = Ξ“ =

For Ξ“(<<Ξ”), optimum Ξ² is Ξ²=0.2 – 1.

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Ξ“ = Ξ“ =

Rs as functions of Ξ² for different T

Ξ“ = Ξ“ =

For Ξ“(<<Ξ”), optimum Ξ² is Ξ²=0.2 – 1. Taking d=1nm, Ξ²<1 corresponds to RB< 1.8*10-14Ξ©m2

This is two orders of magnitude smaller than the lowest contact resistance of YBCO/Ag [J. W. Ekin et al., Appl. Phys. Lett. 62, 369 (1993)]

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Surface Resistance

Bulk magnetic impurities

We will ill see bro roadening of f DOS peak du due to magnetic im impurit itie ies ca can al also re reduce Rs.

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We use the quasiclassical theory in the diffusive limit (Usadel eq.).

Magnetic impurities

Ξ“π‘ž = ℏ𝑀𝐺 2β„“π‘ž

β„“π‘ž : mean spacing of magnetic impurities

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We use the quasiclassical theory in the diffusive limit (Usadel eq.).

Magnetic impurities

Ξ“π‘ž = ℏ𝑀𝐺 2β„“π‘ž

β„“π‘ž : mean spacing of magnetic impurities Ξ“

π‘ž

Ξ” = 0.001

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We use the quasiclassical theory in the diffusive limit (Usadel eq.).

Magnetic impurities

Ξ“π‘ž = ℏ𝑀𝐺 2β„“π‘ž

β„“π‘ž : mean spacing of magnetic impurities Ξ“

π‘ž

Ξ” = 0.001 Ξ“

π‘ž

Ξ” = 0.02

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The surfa face re resis istance can be re reduced by an appropriate density of magnetic impurities!

π‘™π‘ˆ βˆ† =

Ξ“π‘ž Ξ” ~0.01 corresponds to the mean spacing of

magnetic impurities ℓ𝒒~ π„πŸ

𝟏.𝟏𝟐 ~ 4μm

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Summary

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 The main broadening effect can occur in a layer much thinner than πœ‡: DOS in the bulk can be much sharper than the surface.  Tunneling surface probes such as STM do not give all information about DOS in x ≲ πœ‡.  Fitting the tunneling data of DOS with Dynes formula and extracting Ξ“ to describe the low-T surface impedance Z can be misleading. A combination of tunneling measurement and Z in a sufficiently broad T range may offer a possibility to separate the surface and bulk contributions.

Summary

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 A thin pairbreaking layer or a weakly-coupled normal layer at the surface can radically (by orders of magnitude) increase Ri as compared to an ideal surface with only bulk broadening mechanisms.  However, Rs(T) can be reduced by optimizing DOS at the surface by tuning the properties of a proximity-coupled N layer at the surface. [β<1 corresponds to RB< 1.8*10-14Ωm2 for Nb with d=1nm normal layer]

Summary (cont.)

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 Introducing a tiny density of magnetic impurities (ℓ𝒒~ΞΌm for Nb) leads to moderator broaden DOS and reduces Rs.

Summary (cont.)

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Backup Units of temperature and surface resistance for Nb case

𝑆1 = 𝜈0

2πœ‡3πœ•Ξ”

2β„πœπ‘‘ ~10βˆ’4Ξ© 𝑆1 = 𝜈0

2πœ•2πœ‡2πœŠπ‘‘

2πœπ‘‘ ~10βˆ’7Ξ© π‘™πΆπ‘ˆ βˆ† β‰ˆ π‘ˆ 17.5K

(Slide 48) (Slide 59)