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Molten Salt Reactor Workshop 2017 Key Technology and Safety Issues for MSRs October 3 - 4, 2017 Natural Circulation Salt Heat Transfer X. Sun, H.C. Lin, and S. Zhang Department of Nuclear Engineering and Radiological Sciences University of


  1. Molten Salt Reactor Workshop 2017 Key Technology and Safety Issues for MSRs October 3 - 4, 2017 Natural Circulation Salt Heat Transfer X. Sun, H.C. Lin, and S. Zhang Department of Nuclear Engineering and Radiological Sciences University of Michigan Session 7: Support for Salt Technologies 10/04/2017

  2. Prandtl Number of Different Fluids • Liquid Salts - FLiBe - FLiNaK - KF-ZrF 4 - KCl-MgCl 2 - KNO 3 -NaNO 2 -NaNO 3 • Water • Dowtherm A • Air 2

  3. � Natural/Forced Convection Heat Transfer Coefficient Correlations Natural Correlation Geometry Working Pr range Ra or Re Ref. Convection fluid range (NC)/Forced Convection (FC) Ra ≤ 10 /8 NC Vertical plate Sodium, 0.004 ≤ Pr ≤ 300 [1] Nu mercury, = 0.825 air, water, ⁄ 0.387Ra / 0 + oil 7 89 ⁄ ⁄ 6 /0 1 + 0.437 Pr 10 < ≤ Ra ⁄ NC Nu = 0.54Ra / ; Horizontal plate, Air Pr = 0.7 [2] ≤ 2×10 9 hot surface facing up ⁄ 3×10 < NC Nu = 0.27Ra / ; Horizontal plate, Air Pr = 0.7 hot surface ≤ Ra ≤ 10 /? facing down Nu = 0.474Ra ?.8< P𝑠 ?.?;9 3×10 8 NC Horizontal Air, water, 0.7 ≤ Pr ≤ 3090 [3] cylinder silicone ≤ Ra ≤ 2×10 9 oils 3

  4. Natural/Forced Convection HTC Correlations (Cont’d) Natural Correlation Geometry Working Pr range Ra or Re Ref. Convection fluid range (NC)/Forced Convection (FC) Ra ≤ 10 // NC Nu Spheres air, water, oil Pr ≥ 0.7 [4] ⁄ 0.589Ra / ; = 2 + ; 6 ⁄ ⁄ 6 /0 1 + 0.469 Pr Re ≥ 10 ; FC Nu Pipe air, water, oil 0.7 ≤ Pr [5] = 0.027Re ?.7 Pr / E ⁄ ?./; ⁄ ≤ 16700 𝜈 𝜈 G FC Pipe air, water, oil 0.7 ≤ Pr Re [6] / E ⁄ 𝐸 ⁄ Pr / E Nu = 1.86Re / E ⁄ ≤ 16700 ≤ 2300 𝑀 ?./; ⁄ 𝜈 𝜈 G FC Nu Pipe air, water, oil 0.7 ≤ Pr ≤ 3 3500 [7] ⁄ ≤ Re = 0.116JRe 8 E ≤ 1.2 − 125LPr / E ⁄ ?./; ⁄ 𝜈 𝜈 G ×10 ; 4

  5. Natural/Forced Convection HTC Correlations (Cont’d) Natural Correlation Geometry Working Pr range Ra or Re Ref. Convection fluid range (NC)/Forced Convection (FC) Nu = 0.023Re ?.7 P𝑠 M Re ≥ 10 ; FC Pipe air, water, 0.7 ≤ Pr ≤ 100 [8] 𝑜 = 0.4 if the fluid is heated oil 𝑜 = 0.3 if the fluid is cooled Re ≤ 7.6×10 ; FC Nu Sphere air, water, 0.7 ≤ Pr ≤ 380 [9] = 2 oil + J0.4Re ?.< ⁄ LPr ?.; + 0.06Re 8 E Re ≥ 10 ; Nu = 0.023Re ?.7 Pr / E ⁄ FC Pipe air, water, 0.7 ≤ Pr ≤ 100 [10] oil 5

  6. Comparison of Colburn Correlation with Salt Forced Circulation Experiments (G. Yoder, 2014) 6

  7. Comparison with Salt Forced Circulation Experiments +20% -20% Sieder Tate correlation for trubulent flow: ⁄ Nu = 0.027Re ?.7 Pr / E ⁄ ?./; 𝜈 𝜈 G Sieder Tate correlation for laminar flow: ⁄ / E 𝐸 ⁄ Pr / E ⁄ Nu = 1.86Re / E ?./; 𝜈 𝜈 G ⁄ 𝑀 Hausen correlation for transitional flow: ⁄ − 125 Pr / E Nu = 0.116 Re 8 E ⁄ ?./; 𝜈 𝜈 G ⁄ 7

  8. Thermal Expansion Coefficient for Different Fluids • FLiBe • FLiNaK • KF-ZrF 4 • KCl-MgCl 2 • H 2 O (1 atm) ( ) g Δ h Δ p = ρ 0 β Δ T 8

  9. Review of Natural/Forced Circulation Loops for MSRs/FHRs at max Organization NC/FC Experiment Objective Material Working fluid Max Max Ref. Modeling working temp. power temp. (K -1 ) (kW) ( o C) Oak Ridge NC Experiment Preparation for operation of the MSRE Hastelloy N LiF-BeF 2 -ZrF 4 -UF 4 , 784 -- 30,000 [11] National Single loop Laboratory, LiF-BeF 2 -ZrF 4 670 8.8 USA a) Determine if the experimental 0.00032 0.5 NC Experiment Nickel FLiNaK 700 [12] Fluent configuration provides sufficient salt crucible [13] velocity for collection of corrosion data; b) Quantify natural circulation salt velocities using a laser Doppler velocimeter; FC Experiment a) Develop a nonintrusive, inductive Inconel 200 heating technique 600 single b) Measure heat transfer characteristics loop 0.00061 2 The Ohio NC Experiment Examine the couplings among the SS 304 Water 76.5 [14] State Relap5 MOD 4.0 natural circulation/convection loops and coupled [15] University provide experience for high-temperature loops (University DRACS loop design of NC Experiment Investigate DRACS performance under SS 316 FLiNaK 722 0.00032 70 Michigan), steady-state and transient conditions, coupled USA including startup, pump trip test w/o IHX loops 9

  10. Review of Natural/Forced Circulation Loops for MSRs/FHRs (Cont’d) at max Organization FC/NC Experiment Objective Material Working fluid Max Max Ref. Modeling working temp. power temp. (K -1 ) (kW) ( o C) University of NC/FC Experiment Provide experimental validation data for Stainless Dowtherm A 120 0.00075 10 [16] California, Relap5-3D system-level thermal hydraulic codes; steel/copper [17] Berkeley, modeling Serve as an advanced reactor test bed; USA University of NC/FC Experiment System code validation; Heat exchanger Stainless Dowtherm A -- -- 20 [18] New Mexico, testing steel USA single loop University of NC Experiment Research in natural circulation stability, -- FLiBe 800 0.00027 -- [19] Wisconsin, Fluent salt freezing, etc. USA FC Experiment Identify salt corrosion and heat transfer SS 316 KCl-MgCl 2 600 0.00029 4 [20] issues Single loop US Industry NC/FC Experiment Gaining operation experience with salts, Salts corrosion, component testing, instrumentation, etc. Ulsan NC Experiment Understand the thermal-hydraulic SS 304 Dowtherm RP 80 0.00071 0.3 [21] National MARS code characteristics of molten salts using Single loop Institute of modeling simulants Science and Technology, Korea 10

  11. Review of Natural/Forced Circulation Loops for MSR/FHR (Cont’d) at max Organization NC/FC Experiment Objective Material Working fluid Max Max Ref. Modeling working temp. power temp. (K -1 ) (kW) ( o C) Shanghai NC Experiment Gather experience on design and SS 316 KNO 3 -NaNO 2 - 450 0.00075 -- [22] Institute of validation of passive decay heat removal Single loop NaNO 3 Applied system for FHRs Physics, FC Experiment Validate system design; Develop Hastelloy FLiNaK 650 0.00032 150 China principle prototypes of molten salt C276 pump, valves, HX, etc. Single loop Beijing NC Experiment Investigate natural circulation heat SS 316 Ca(NO 3 ) 2 - KNO 3 - 250 -- 0.3 [23] University of transfer of molten salt in a single energy tank NaNO 3 -LiNO 3 Technology, storage tank China Bhabha NC Experiment Investigate thermal hydraulics, Inconel 625 KNO 3 -NaNO 3 - 580 0.0006 2 [24] Atomic In-house instrument development, and material Single loop LiNO 3 Research developed related issues relevant to high- Centre, India code temperature reactor, such as MSBR LeBENC Experiments: NC Experiment Hastelloy N LiF-ThF 4 750 0.00049 1 [25] a) Steady-state at different power levels; OpenFOAM Single loop b) Startup transient; c) Loss of heat sink; d) Heater trip; d) Step change in heater power. 11

  12. Review of Natural/Forced Circulation Loops for MSR/FHR (Cont’d) at max Organization NC/FC Experiment Objective Material Working fluid Max Max Ref. Modeling working temp. power temp. (K -1 ) (kW) ( o C) EU project FC Experiment Preparation for MSFR -- FLiNaK 700 0.00032 -- [26] SAMOFAR FFFFER: Forced Fluoride Flow for [27] Experimental Research FC Experiment Study the solidification phenomena of a molten salt Czech FC Experiment Experimental program in MSR physics -- FLiBe -- -- -- [28] Republic and corrosion flow loop 12

  13. Bhabha Atomic Research Centre’s NC Experiments • Startup Startup of natural circulation at 1200 W (A.K. Srivastava, et al., 2016) (A.K. Srivastava, et al., 2016) 13

  14. Heat Transfer Correlations (HTC) in RELAP5 • Define the geometry of heat structure • For single phase liquid, RELAP5 calculate three heat transfer coefficients - find the maximum heat transfer coefficient - ℎ = 𝑛𝑏𝑦 ℎ defgMeh , ℎ jkhlkdmMj , ℎ Mejkhed User defined geometries Laminar Turbulent Natural Standard Dittus-Boelter Churchill-Chu or McAdams Horizontal annuli, flow in plate Dittus-Boelter McAdams and single tube Parallel flow in vertical bundle Dittus-Boelter- Churchill-Chu or McAdams Nu with in-line and staggered rods Inayatov = 4.36 Crossflow in vertical bundle with Dittus-Boelter Churchill-Chu or McAdams in-line and staggered rods Inayatov-Shah Parallel flow and crossflow in horizontal bundle Dittus-Boelter Churchill-Chu with in-line and staggered rods 14

  15. HTC for Flow in Circular Tubes in RELAP5 (Cont’d) • Laminar forced convection (Sallers) - 𝑂𝑣 = 4.36 • Turbulent forced convection (Dittus-Boelter) - 𝑂𝑣 = 0.023𝑆𝑓 ?.7 𝑄𝑠 ?.; • Natural convection (Churchill-Chu) 8 t ?.E79se u - 𝑂𝑣 = 0.825 + } y z~ /v w.xyz tu {| - 𝑆𝑏 = 𝐻𝑠 € Pr 𝐻𝑠 = • z ‚ƒ „ … †„ ‡ ˆ ‰ Š z • Natural convection (McAdams) - 𝑂𝑣 = 0.27𝑆𝑏 ?.8< 15

  16. HTC in TRACE • For single-phase liquid , also take maximum values among laminar and turbulent forced convection and natural convection (NC). - ℎ = 𝑛𝑏𝑦 ℎ defgMeh , ℎ jkhlkdmMj , ℎ defgMeh ‹Œ , ℎ jkhlkdmMj ‹Œ • Geometries - Tube - Rod bundle - Helical Coil - Cross Flow 16

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